Daniel Day Lewis in most of his Films...Gangs of New York comes to mind
As does Little Bill Daggett, played by Gene Hackman in Unforgiven
Hitman Anton Chigurh (Javier Bardem) in No Country for Old Men was intense
The dude from Zodiac was also in the same vein as Bardem, but of course we never got to find out who he was...his tying up of that couple by the lake and then stabbing them was the work of a sick heinous man.
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